Tangier is nice, but I don't think you'd need more than 3 days there unless you really enjoy smoking hash and sitting around drinking mint tea and not doing much of anything. I was there for 5 days this summer, and it was definitely more time than I needed. If you do go, make sure you eat at Le Saveur du Poisson. It was one of the better seafood meals I've ever had, and it wasn't expensive at all.
I haven't been anywhere else in Morocco, but I'd think it could be worth splitting a week between Tangier an Marrakech or Casablanca.
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