The two that come to mind for me right off the bat are Super Mario World and Portal 2. I actually like Portal 1 more, but it's more of a proof of concept, 2 is a much fuller game. Super Mario World's controls still feel so damn good when I pick it up, in my mind it's still the best platformer ever made.
Another one that comes to mind is A Link to the Past, although I do think it's got some small warts that prevent it from being "perfect". People bring up Mega Man X too, but I can't comment on that one as I never played it.
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