I have been practically everywhere in Croatia. Zadar is probably my favourite coastal city there.
Some other places that are a little off the radar are Rovinj, Sibenik, and Korcula.
Having said that, if you are only going once and want to pack as much in as possible, Zagreb, Split, and Dubrovnik are the main staples for most people. They are the places with probably the most touristy things to do and have the most amenities.
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