I'm a huge Tom Petty fan, so I'll list a few that aren't necessarily in his greatest hits catalogs (at least in their studio versions):
Tom Petty
Melinda
It's Good to be King (from the live Anthology - 12 minute version)
Honey Bee
To Find a Friend
Something Good Coming
Christmas All Over Again
I could go on forever with Petty/Wilburys/Mudcrutch, but if you're looking for a bit of a deeper cut, definitely check out Melinda and SNL performance of Honey Bee with Dave Grohl on drums.
Built To Spill
I Would Hurt a Fly
Big Dipper
Goin' Against Your Mind
Mess With Time
Car
Time Trap
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