He has some really good performances from when he was younger.
Charlie Bartlett - He plays a kid reselling the drugs his therapist prescribes to him to his prep-school mates. Opposite Robert Downey Jr.
Alpha Dog - This movies is pretty meh, but Yelchin is excellent in it.
Odd Thomas - I saw this recently, I guess it's based on a book. It's pretty cool. He's a kid who can see how people will die and the spirits that haunt them. I'd recommend.
He was always rumored for Spiderman roles. I wish he had played him at some point.
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