I have no idea if it's "best" or not, but I find Value Village to be the easiest/most convenient for the wife & I. The one in Mindapore is just a matter of rolling up to the back door and dropping stuff off, the kids working there are great about grabbing stuff from your vehicle & the whole thing takes less than 30 seconds most times.
Not sure if 'best' from a charity aspect, but as far as getting rid of stuff it's pretty easy.
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