Patrick Stewart as Prof X. That man was born to play him.
Keaton as Batman. Everyone laughed when this was first announced but he did an excellent job I thought. Right up there with Bale's performance, only Bale had the better scripts and directors and cast etc.
Keanu Reeves in the Matrix. The guy can't act his way out of a paper bag, but can you really imagine anyone else pulling off "Whoa" as well as he did?
Chuck Heston in the Ten Commandments. He was born to play Moses.
The guy who played J. Jonah Jameson in the Spidey movies. He captured what I thought was going to be an untransferable character.
Kevin Spacey in The Usual Suspects.
Anything with Peter Sellers, especially The Party and the Pink Panther movies.
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