I'm not a huge fan of episodic anime, I easily prefer long story arcs that are the main focus.
I quite enjoyed Death Note and Code Geass for that...really enjoyed Attack on Titan as well.
A shout out for Legend of the Galactic Heroes as well. I didn't quite finish it but I came close...didn't pick it up again after a sad part near the end, but it was very good up to that point.
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